ToughMOF: Tailoring Metal-Organic Framework Glasses with Higher Fracture Toughness

Research output

Research output per year 2021 2022 2023 2024 2024

• 18 Journal article
• 12 Conference abstract for conference
• 1 Poster

Research output per year

Research output per year

Search results

• 2024

  Constructing artificial metal-organic framework glass layer to regulate lithium plating and stripping

  Ding, J., Du, T. & Smedskjær, M. M., 12 Mar 2024.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research

  File

  • Plating 100%
  • Lithium 100%
  • Metal-Organic Framework 100%
  • Battery (Electrochemical Energy Engineering) 100%
  • Glass Layer 100%
  28 Downloads (Pure)

• Deciphering the controlling factors for phase transitions in zeolitic imidazolate frameworks

  Du, T., Li, S., Ganisetti, S., Bauchy, M., Yue, Y. & Smedskjær, M. M., Apr 2024, In: National Science Review. 11, 4, 13 p., nwae023.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Crystalline Material 100%
  • Metal-Organic Framework 100%
  • Amorphous Material 100%
  • Structure 100%
  • Vitrification 50%
  4 Citations (Scopus)

  19 Downloads (Pure)

• Enhanced bond switching at complexion layer facilitates high fracture energy of LATP solid-state electrolytes

  Chen, Z., Du, T., Krishnan, N. M. A. & Smedskjær, M. M., 2024, In: Journal of Materials Chemistry A. 12, 5, p. 3061-3071 11 p.

  Research output: Contribution to journal › Journal article › Research › peer-review

  File

  • Solid Electrolyte 100%
  • Glass Ceramics 100%
  • Li1.3Al0.3Ti1.7(PO4)3 100%
  • Mechanical Property 66%
  • Fracture Behavior 33%
  2 Citations (Scopus)

  16 Downloads (Pure)

• High-performance dendrite-free lithium metal anode based on metal-organic framework glass

  Ding, J., Du, T., Jensen, L. R., Sørensen, S. S., Wang, D., Wang, S., Zhang, L., Yue, Y. & Smedskjær, M. M., 18 Jul 2024, In: Advanced Materials. 36, 29, 2400652.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Dendrite-Free 100%
  • Lithium Metal Anode 100%
  • Glass Layer 100%
  • Metal-Organic Framework 100%
  • Dendrite-free Anodes 100%
  1 Citation (Scopus)

  17 Downloads (Pure)

• Metal-Organic Framework Glass as a Functional Filler Enables Enhanced Performance of Solid-State Polymer Electrolytes for Lithium Metal Batteries

  Ding, J., Du, T., Thomsen, E. H., Andresen, D., Fischer, M. R., Møller, A. K., Petersen, A. R., Pedersen, A. K., Jensen, L. R., Wang, S. & Smedskjær, M. M., Mar 2024, In: Advanced Science. 11, 10, 2306698.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Polymer Electrolyte 100%
  • Metal-Organic Framework 100%
  • Lithium Metal Battery 100%
  • Ionic Liquid 80%
  • Polyethylene Glycol 40%
  5 Citations (Scopus)

  31 Downloads (Pure)

• Structural descriptors for zeolitic imidazolate framework glasses

  Smedskjær, M. M., 22 May 2024.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File
  22 Downloads (Pure)

• Structural Origin of the Deformation Propensity of Zeolitic Imidazolate Framework Glasses

  Du, T., Ge, X., Cao, F., Liu, H., Shi, C., Ding, J., Sun, D., Zhang, Q., Yue, Y. & Smedskjaer, M. M., 25 Jun 2024, In: Chemistry of Materials. 36, 12, p. 6167-6179 13 p.

  Research output: Contribution to journal › Journal article › Research › peer-review

  • Fracture Toughness 100%
  • Glass Composition 100%
  • Catalysis 100%
  • Young's Modulus 100%
  • Metal-Organic Framework 100%
  1 Citation (Scopus)

• Toughening mechanism of barium titanosilicate glass-ceramics

  Sun, D., Du, T., Zhang, Q., Jensen, L. R., Wang, D., Ding, J., Zhao, J. & Smedskjær, M. M., Oct 2024, In: Materials & Design. 246, 113303.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Glass-ceramics 100%
  • Barium 100%
  • Toughening Mechanism 100%
  • Titanosilicate 100%
  • Glass Ceramics 100%
  8 Downloads (Pure)
• 2023

  Controlling factor for fracture resistance and ionic conduction in glassy lithium borophosphate electrolytes

  Du, T., Chen, Z., Liu, H., Zhang, Q., Bauchy, M., Yue, Y. & Smedskjær, M. M., Oct 2023, In: Materials Today Energy. 37, 101390.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Fracture Toughness 100%
  • Lithium 100%
  • Ionic Conductivity 100%
  • Ionic Conduction 100%
  • Solid Electrolyte 50%
  3 Citations (Scopus)

  52 Downloads (Pure)

• Deciphering How Anion Clusters Govern Lithium Conduction in Glassy Thiophosphate Electrolytes through Machine Learning

  Chen, Z., Du, T., Christensen, R., Bauchy, M. & Smedskjær, M. M., 14 Apr 2023, In: ACS Energy Letters. 8, 4, p. 1969–1975 7 p.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Thiophosphate Solid Electrolyte 100%
  • Lithium Ion Migration 100%
  • Anion Cluster 100%
  • Li2S-P2S5 100%
  • Lithium 100%
  5 Citations (Scopus)

  15 Downloads (Pure)

• Deciphering the hierarchical structure of phosphate glasses using persistent homology with optimized input radii

  Xiao, Y., Du, T., Sørensen, S. S., Chen, Z., Biscio, C., Fajstrup, L., Bauchy, M. & Smedskjær, M. M., 29 Jun 2023, In: Physical Review Materials. 7, 6, 065602.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Range Order 100%
  • Phosphate Glass 100%
  • Homology 100%
  • Medium-Range Order 100%
  • Vertex Weight 75%
  2 Citations (Scopus)

  5 Downloads (Pure)

• Decoding Structure-Property Relations in Oxide Glasses Using Classification-Based Machine Learning

  Du, T., Bauchy, M. & Smedskjær, M. M., 2023.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File
  13 Downloads (Pure)

• High damage-resistance and fracture toughness of transparent Nb-doped barium aluminoborate glass ceramics

  Zhang, Q., Sun, D., Du, T., Jensen, L. R., Wang, D., Popok, V., Youngman, R. E. & Smedskjær, M. M., Oct 2023, In: Applied Materials Today. 34, 101888.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Crack Initiation 100%
  • Fracture Toughness 100%
  • Barium 100%
  • Glass Ceramics 100%
  • Damage Fracture 100%
  4 Citations (Scopus)

  61 Downloads (Pure)

• Irradiation of Zeolitic Imidazolate Framework Crystals and Glasses: A Molecular Dynamics Study

  Du, T., Sørensen, S. S., Zhou, Q., Bauchy, M. & Smedskjær, M. M., 2023.

  Research output: Contribution to conference without publisher/journal › Poster › Research › peer-review

  File
  10 Downloads (Pure)

• Predicting Fracture and Conduction Propensity in Glassy Electrolytes Using Classification-Based Machine Learning

  Du, T., Chen, Z., Bauchy, M., Yue, Y. & Smedskjær, M. M., 2023.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  Open Access

  File
  50 Downloads (Pure)

• Structure dependence of fracture toughness and ionic conductivity in lithium borophosphate glassy electrolytes for all-solid-state batteries

  Chen, Z., Du, T., Sørensen, S. S., Christensen, R., Zhang, Q., Jensen, L. R., Magdysyuk, O. V., Diaz-Lopez, M., Bauchy, M., Yue, Y. & Smedskjær, M. M., 1 Jan 2023, In: Journal of Power Sources. 553, 232302.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Fracture Toughness 100%
  • Borophosphate Glass 100%
  • Lithium 100%
  • Lithium Ion 100%
  • Ionic Conductivity 100%
  6 Citations (Scopus)

  139 Downloads (Pure)

• Understanding the Structure and Mechanical Properties of ZIF Glasses by a Machine Learning Force Field

  Du, T., Yue, Y. & Smedskjær, M. M., 2023.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File
  57 Downloads (Pure)

• Water as a Modifier in a Hybrid Coordination Network Glass

  Sørensen, S. S., Ren, X., Du, T., Traverson, A., Xi, S., Jensen, L. R., Bauchy, M., Horike, S., Wang, J. & Smedskjær, M. M., 5 Apr 2023, In: Small. 19, 14, 2205988.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Glass Transition Temperature 100%
  • Oxide Glass 100%
  • Glass Composition 100%
  • Cobalt 100%
  • Transition Metal 100%
  3 Citations (Scopus)

  50 Downloads (Pure)
• 2022

  Accessing a Forbidden Disordered State of a Zeolitic Imidazolate Framework with Higher Stiffness and Toughness through Irradiation

  Du, T., Sørensen, S. S., Zhou, Q., Bauchy, M. & Smedskjær, M. M., 20 Sept 2022, In: Chemistry of Materials. 34, 19, p. 8749-8759 11 p.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Metal-Organic Framework 100%
  • Catalysis 20%
  • Silicate 20%
  • Structural Disordering 20%
  • Silicate Minerals 20%
  9 Citations (Scopus)

  52 Downloads (Pure)

• Correlating Structure with Mechanical Properties in Hybrid Glasses: Invited Talk

  Smedskjær, M. M., 5 Jul 2022.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File
  23 Downloads (Pure)

• Disordering of Metal-Organic Framework Crystals and Glasses upon Irradiation

  Du, T., Sørensen, S. S., Bauchy, M. & Smedskjær, M. M., 8 Jul 2022.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File

  • Metal-Organic Framework 100%
  • Disordered State 40%
  • Vitrification 33%
  • Disordered Metals 20%
  18 Downloads (Pure)

• Fracture and Bond Switching in Simulated Glassy Alumina and Silica

  Smedskjær, M. M. & Du, T., 23 May 2022.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File
  36 Downloads (Pure)

• Glass Irradiation: Impact on Structure and Mechanical Properties

  Smedskjær, M. M., Du, T. & Ren, X., 24 May 2022.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File
  44 Downloads (Pure)

• Irradiation-induced toughening of calcium aluminoborosilicate glasses

  Ren, X., Du, T., Peng, H., Jensen, L. R., Biscio, C., Fajstrup, L., Bauchy, M. & Smedskjær, M. M., Jun 2022, In: Materials Today Communications. 31, 103649.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Fracture Toughness 100%
  • Surface Defect 33%
  • Crack Initiation 33%
  • Boron 33%
  • Coarsening 33%
  8 Citations (Scopus)

  67 Downloads (Pure)

• Oxide glasses under pressure: Recent insights from experiments and simulations

  Du, T., Sørensen, S. S., To, T. & Smedskjær, M. M., 2 May 2022, In: Journal of Applied Physics. 131, 17, 170901.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Overpressure 100%
  • Oxide Glasses 100%
  • Oxide Glass 100%
  • Densification 60%
  • Structural Change 20%
  13 Citations (Scopus)

  92 Downloads (Pure)

• Persistent homology: A tool to understand medium-range order glass structure

  Sørensen, S. S., Du, T., Biscio, C., Fajstrup, L. & Smedskjær, M. M., Dec 2022, In: Journal of Non-Crystalline Solids: X. 16, 100123.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Medium-Range Order 100%
  • Coordination Shell 33%
  • Atomic Position 33%
  12 Citations (Scopus)

  214 Downloads (Pure)

• Predicting Bond Switching and Fracture in Simulated Al2O3 Glass Using Machine Learning

  Du, T., Liu, H., Tang, L., Sørensen, S. S., Bauchy, M. & Smedskjær, M. M., 6 Jul 2022.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File

  • Al2O3 100%
  • Strained Structures 50%
  • High Strain Rate 50%
  • Strain Rate 33%
  • Oxide Glass 33%
  22 Downloads (Pure)

• Resolving the Conflict between Strength and Toughness in Bioactive Silica–Polymer Hybrid Materials

  Fan, W., Du, T., Droce, A., Jensen, L. R., Youngman, R. E., Ren, X., Gurevich, L., Bauchy, M., Kristensen, P., Xing, B., Yu, D. & Smedskjær, M. M., 9 Jun 2022, In: ACS Nano. 16, 6, p. 9748–9761 14 p.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Hybrid Material 100%
  • Mechanical Strength 100%
  • Silicon Dioxide 50%
  • Inorganic Polymer 25%
  • Inorganic Glass 25%
  10 Citations (Scopus)

  65 Downloads (Pure)

• Water as a flux in a hybrid coordination network glass

  Sørensen, S. S., Ren, X., Du, T., Jensen, L. R. & Smedskjær, M. M., 23 May 2022.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File
  47 Downloads (Pure)
• 2021

  Fracture Toughness of Zeolitic Imidazolate Framework Glasses: Invited Talk

  Smedskjær, M. M., To, T., Sørensen, S. S., Du, T., Yue, Y. & Bauchy, M., 2021.

  Research output: Contribution to conference without publisher/journal › Conference abstract for conference › Research › peer-review

  File
  59 Downloads (Pure)

• Predicting Fracture Propensity in Amorphous Alumina from Its Static Structure Using Machine Learning

  Du, T., Liu, H., Tang, L., Sørensen, S. S., Bauchy, M. & Smedskjær, M. M., 23 Nov 2021, In: ACS Nano. 15, 11, p. 17705-17716 12 p.

  Research output: Contribution to journal › Journal article › Research › peer-review

  Open Access

  File

  • Al2O3 100%
  • Amorphous Material 100%
  • Aluminum Oxide 100%
  • α-Al2O3 100%
  • Amorphous Alumina 100%
  25 Citations (Scopus)

  107 Downloads (Pure)