Abstract
The accumulation of microplastics (MPs) in the sediments of a stormwater treatment pond was studied to gain knowledge on how these facilities protect the natural environment against this emerging pollutant. Thirteen sediment samples were analyzed for MPs down to 10 μm, mapping the pattern of accumulation in the pond. The average abundance in terms of MP-number and mass was 11.8 μg kg−1 and 44,383 item kg−1, respectively. They were rather unevenly distributed, with concentrations varying up to two orders of magnitude within the pond, showing that a trustworthy quantification of MPs retained by such units must rely on many and well-distributed subsamples. Buoyant MPs made up 95.4 % of the MP-mass and 83.5 % of the MP-number and in most of the sampled locations, polypropylene dominated the polymer fingerprint, followed by polyethylene. No spatial pattern in the distribution of MPs in the pond was identified. Instead, the MP content correlated to the organic matter and silt content, indicating that the processes leading to deposition could be similar. A computational fluid dynamics model was set up and used to simulate the transport mechanisms governing the conveyance of MPs in the pond from water to sediments. The results showed that the combination of advection and dispersion were likely the driving mechanism for buoyant (and non-buoyant) MPs to get in contact with the sediment bed and spread over the pond. Once in contact with the sediments, the MPs would have some probability of being permanently incorporated and hereby preventing them from entering the downstream aquatic environment.
Original language | English |
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Article number | 160489 |
Journal | Science of the Total Environment |
Volume | 860 |
ISSN | 0048-9697 |
DOIs | |
Publication status | Published - 20 Feb 2023 |
Bibliographical note
Funding Information:This work was carried out within the Limnoplast project. This project has received funding from the European Union’s Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie grant agreement No 860720 .
Funding Information:
This work was carried out within the Limnoplast project. This project has received funding from the European Union's Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie grant agreement No 860720.
Publisher Copyright:
© 2022 The Authors
Keywords
- Buoyant MPs
- CFD
- Sediments
- Stormwater ponds