Excitonic magneto-optics in monolayer transition metal dichalcogenides: From nanoribbons to two-dimensional response

Jonas Have, N.M.R. Peres, Thomas Garm Pedersen

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Abstract

The magneto-optical response of monolayer transition metal dichalcogenides, including excitonic effects, is studied using a nanoribbon geometry. We compute the diagonal optical conductivity and the Hall conductivity. Comparing the excitonic optical Hall conductivity to results obtained in the independent-particle approximation, we find an increase in the amplitude corresponding to one order of magnitude when excitonic effects are included. The Hall conductivities are used to calculate Faraday rotation spectra for MoS2 and WSe2. Finally, we have also calculated the diamagnetic shift of the exciton states of WSe2 in different dielectric environments. Comparing the calculated diamagnetic shift to recent experimental measurements, we find a very good agreement between the two.

Original languageEnglish
Article number045411
JournalPhysical Review B
Volume100
Issue number4
Number of pages10
ISSN2469-9950
DOIs
Publication statusPublished - 15 Jul 2019

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