A binder-free Si-based anode for Li-ion batteries

Chunqian Zhang; Fan Yang; Dalin Zhang; Xu Zhang; Chunlai Xue; Yuhua Zuo; Chuanbo Li; Buwen Cheng; Qiming Wang

doi:10.1039/c4ra15159c

A binder-free Si-based anode for Li-ion batteries

Chunqian Zhang, Fan Yang, Dalin Zhang, Xu Zhang, Chunlai Xue, Yuhua Zuo, Chuanbo Li^*, Buwen Cheng, Qiming Wang

^*Corresponding author for this work

Research output: Contribution to journal › Journal article › Research › peer-review

16 Citations (Scopus)

Abstract

A binder-free anode for lithium ion batteries consisting of micro-sized silicon particles and polyacrylonitrile (PAN) was prepared. By optimizing the size of the Si particles and the ratio of Si particles to PAN, the performance of the anode was greatly enhanced. Although its columbic efficiency in the first cycle is comparatively lower than that made by traditional methods, it increases to 99% in the 8th cycle, and remains above 99.5% for up to 190+ cycles. Due to its adhesivity and conductance, pyrolyzed PAN (PPAN) can be used both as a binder and the conductive agent at the same time.

Original language	English
Journal	RSC Advances
Volume	5
Issue number	21
Pages (from-to)	15940-15943
Number of pages	4
ISSN	2046-2069
DOIs	https://doi.org/10.1039/c4ra15159c
Publication status	Published - 2015

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© The Royal Society of Chemistry 2015.

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title = "A binder-free Si-based anode for Li-ion batteries",

abstract = "A binder-free anode for lithium ion batteries consisting of micro-sized silicon particles and polyacrylonitrile (PAN) was prepared. By optimizing the size of the Si particles and the ratio of Si particles to PAN, the performance of the anode was greatly enhanced. Although its columbic efficiency in the first cycle is comparatively lower than that made by traditional methods, it increases to 99% in the 8th cycle, and remains above 99.5% for up to 190+ cycles. Due to its adhesivity and conductance, pyrolyzed PAN (PPAN) can be used both as a binder and the conductive agent at the same time.",

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T1 - A binder-free Si-based anode for Li-ion batteries

AU - Zhang, Chunqian

AU - Yang, Fan

AU - Zhang, Dalin

AU - Zhang, Xu

AU - Xue, Chunlai

AU - Zuo, Yuhua

AU - Li, Chuanbo

AU - Cheng, Buwen

AU - Wang, Qiming

PY - 2015

Y1 - 2015

N2 - A binder-free anode for lithium ion batteries consisting of micro-sized silicon particles and polyacrylonitrile (PAN) was prepared. By optimizing the size of the Si particles and the ratio of Si particles to PAN, the performance of the anode was greatly enhanced. Although its columbic efficiency in the first cycle is comparatively lower than that made by traditional methods, it increases to 99% in the 8th cycle, and remains above 99.5% for up to 190+ cycles. Due to its adhesivity and conductance, pyrolyzed PAN (PPAN) can be used both as a binder and the conductive agent at the same time.

AB - A binder-free anode for lithium ion batteries consisting of micro-sized silicon particles and polyacrylonitrile (PAN) was prepared. By optimizing the size of the Si particles and the ratio of Si particles to PAN, the performance of the anode was greatly enhanced. Although its columbic efficiency in the first cycle is comparatively lower than that made by traditional methods, it increases to 99% in the 8th cycle, and remains above 99.5% for up to 190+ cycles. Due to its adhesivity and conductance, pyrolyzed PAN (PPAN) can be used both as a binder and the conductive agent at the same time.

UR - http://www.scopus.com/inward/record.url?scp=84922807002&partnerID=8YFLogxK

U2 - 10.1039/c4ra15159c

DO - 10.1039/c4ra15159c

M3 - Journal article

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SN - 2046-2069

VL - 5

SP - 15940

EP - 15943

JO - RSC Advances

JF - RSC Advances

IS - 21

ER -

A binder-free Si-based anode for Li-ion batteries

Abstract

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